Quantification of the heterogeneity of particle packings

Schenker, Iwan and Filser, Frank and Gauckler, Ludwig and Aste, T. and Herrmann, Hans (2009) Quantification of the heterogeneity of particle packings. Physical Review E, 80 (2). ISSN 1539-3755. (Full text available)

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http://dx.doi.org/10.1103/PhysRevE.80.021302

Abstract

The microstructure of coagulated colloidal particles, for which the interparticle potential is described by the Derjaguin-Landau-Verweg-Overbeek theory, is strongly influenced by the particles’ surface potential. Depending on its value, the resulting microstructures are either more “homogeneous” or more “heterogeneous,” at equal volume fractions. An adequate quantification of a structure’s degree of heterogeneity (DOH), however, does not yet exist. In this work, methods to quantify and thus classify the DOH of microstructures are investigated and compared. Three methods are evaluated using particle packings generated by Brownian dynamics simulations: (1) the pore size distribution, (2) the density-fluctuation method, and (3) the Voronoi volume distribution. Each method provides a scalar measure, either via a parameter in a fit function or an integral, which correlates with the heterogeneity of the microstructure and which thus allows to quantitatively capture the DOH of a granular material. An analysis of the differences in the density fluctuations between two structures additionally allows for a detailed determination of the length scale on which differences in heterogeneity are most pronounced.

Item Type: Article
Subjects: Q Science
Divisions: Faculties > Science Technology and Medical Studies > School of Physical Sciences > Functional Materials Group
Depositing User: Tomaso Aste
Date Deposited: 20 Mar 2012 16:19
Last Modified: 28 Mar 2012 09:10
Resource URI: http://kar.kent.ac.uk/id/eprint/29173 (The current URI for this page, for reference purposes)
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